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The collection consists primarily of forty-two bound volumes covering Roger Griffin's research and publications from circa 1955 to circa 1991. Topics and publications include observation logs, Observatory Magazine, The Spectroscopic Binaries, Griffin's Fellowship dissertation for St John's, computing, RV reductions, spectroscopy, and radial velocities.

Seven card-index boxes, made by Griffin, contain many years' worth of raw data from radial-velocity spectrometer observations. Digital versions can be viewed at https://www.squarewheels.org.uk/rfg/unpub/ .

There are also notebooks containing material on observations and telescope maintenance, a chart roll of spectrometer output, a 1977 leaflet on the Cambridge North Norway Expedition, and papers on the Cripps development at St John's.

Carbon copies of typescript letters sent by Guest on St John's College choir and other business, papers relating to choir tours, and other miscellaneous correspondence.

Articles, reports, and speeches by Guillebaud, plus cuttings and obituaries.

The papers consist of letters written by Nathaniel to his family during his service in the Boer War, a diary for 1900, and an unpublished autobiography written in and before 1943.

Correspondence, material relating to the Harper-Wood Studentship, poems, Harper's autobiography, typescripts.

Notebooks containing notes on classical subjects and translations; notebook used as Junior Bursar, containing notes on College Council business; diary of a holiday in the Isle of Wight.

Letters and picture (dated 1812-1955), documents relating to Herschel's 1839 paper, 'The Art of Photography', given to the Royal Society, (dated 1833-1979), Herschel's notebooks.

Papers relating to Hiller's army career, letters to family, postcards, photographs and First World War ephemera.

A small quantity of personal and professional papers and medals, given by various sources.

Diaries. Gives details of religious life in Edwardian Cambridge, especially with reference to Anglo-Catholicism. Includes letters to How and printed material regarding church matters.